If I was PAYING $$$ to convert, I would go 4.56 without question. Here's the logic:
The 66RFE transmission gear ratios are the same as the 68RFE. 6th gear is very tall and designed for the Cummins. It's @ .625 OD!
To make a robust 6.4L Transmission, it was a good decision for FCA to just take the same basic 68RFE transmission guts (with a slightly ligher duty torque converter) and put it in a 545RFE case (for easy mating / packaging to the gas engines) and call it the 66RFE.
Here are the ratios:
But 6th gear is really designed for a low rpm / torque monster. The 6.4L HEMI, as great as it is, likes to rev. Even with the 4.56, I don't believe 6th gear will rev too high with this much OD in 6th @ .625:1
I have the 4.10 and I would even like a little higher ratio rear end. I would not bother going any less than the 4.56 if I were spending the money.
Just something to think about...
-Guzzler